Urban skyline is one of the visible attributes that allow us to recognize the position, orientation,and characters of the urban environment. This study aims to establish the quantiative method for describing skylines and the numerical consequence of the formation of skylines. The quantitative study includes two parts:(1) the first part is discuss the observation of skylines; (2) the second parts is to build a quantitative method which utilizes a statistic approach to calculate the variance and dispersion of skylines. The quantitative method simplifies the image of skylines into "bar-mass" charts, measures and analyzes the numerical values of skylines. It is constructed for explaining the interrelationships of the formation of skylines between"the outlines"and "numerical values."The finding indicates that the quantitative method as described in multi-dimensional numerical values will enhance the accuracy and completeness in describing the formation of skylines, and the numerical values presented in analysis will assist the explanation of shaping urban forms. By the accumulation of skyline case studies, it is possible to analyze the regularity of skylines, and provide us to set up the criteria of urban design guidelines for better cityscape from quantitative analysis.