A methodology of assessing the users’ psychological behavior effect is necessary, especially in high-rise building areas. The concept and analysis methods of this study are (1)system analysis method, (2)psychological attitude scale, (3)a law of comparative judgement, (4)pair-wise comparative method, and (5)regression analysis technique. The contents of environmental behavior interaction include the context、property、evaluation、practice and its application. Basing on the results, we can conclude that the physical value does not limit psychological effect value. The psychological effect value should improve the measurement of psychology response scale by the law of comparative judgement and pair-wise comparative method. This article suggests a system analysis process for establishing an interaction models and operation technology which is based on the viewpoints of environmental behavior interactions is high-rise building areas concerning with users' safety, health, efficiency and comfort environment. It provides the planner a valuable reference of environmental planning and design. Moreover, recognizing environmental behavior interactions and directions in the future is discussed as well.