Service-Learning is more and more important in higher education which can help students develop civic consciousness and sense of responsibility, and pre-service training design is very critical to the Service-Learning quality of volunteer teams. The purpose of this study was to explore the relationship between the pre-service training design and the learning satisfaction of Tamkang University current volunteer teams. 248 effective questionnaires are obtained from this population. ANOVA, Pearson product-moment correlation and regression statistical method were adopted in this study. The present result shows that pre-service training design and the Service- Learning satisfaction are significant positive correlative. And the course design of pre-service training is most predictive to the learning satisfaction of interpersonal interactions and social concern.